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Asymmetric Synthesis of Bioactive Lactones and the Development of a Catalytic Asymmetric Synthesis of -Aryl Ketones

Springer Theses

By (author) Robert Doran
Format: Paperback / softback
Publisher: Springer International Publishing AG, Cham, Switzerland
Published: 15th Oct 2016
Dimensions: w 156mm h 234mm d 12mm
Weight: 324g
ISBN-10: 3319370340
ISBN-13: 9783319370347
Barcode No: 9783319370347
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Synopsis
This thesis addresses two fundamental areas in contemporary organic chemistry: synthesis of natural products and catalytic asymmetric synthesis. Firstly, a new methodology, developed by our research group, which allows the asymmetric synthesis of lactones, a structural unit ubiquitous in natural products, was utilised in the synthesis of a number of natural product analogues that showed significant biological activity. Secondly, the development of a catalytic asymmetric synthesis of a key structural motif present in a number of natural products and pharmaceuticals was accomplished. During the course of this work we discovered dual stereo control, which is significant because it allows the configuration of a new stereo centre to be controlled by a simple change of proton source.

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